Abstract

Epidemiological studies suggest that the main part of chronic effects from air pollution is likely to be linked with particulate matter (PM). Oxidative potential (OP) of PM is gaining strong interest as a promising health exposure metric. This study combined atmospheric detailed composition results obtained for seven different urban background environments over France to examine any possible common feature in OP seasonal variations obtained using two assays (acid ascorbic (AA) and dithiothreitol (DTT)) along a large set of samples ( N &gt

700 ). A remarkable homogeneity in annual cycles was observed with a higher OP activity in wintertime at all investigated sites. Univariate correlations were used to link the concentrations of some major chemical components of PM and their OP. Four PM components were identified as OP predictors: OC, EC, monosaccharides and Cu. These species are notably emitted by road transport and biomass burning, targeting main sources probably responsible for the measured OP activity. The results obtained confirm that the relationship between OP and atmospheric pollutants is assay- and location-dependent and, thus, the strong need for a standardized test, or set of tests, for further regulation purposes.

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The different versions of the original document can be found in:

https://hal.archives-ouvertes.fr/hal-02442585/document,
https://hal.archives-ouvertes.fr/hal-02442585/file/atmosphere-10-00698.pdf under the license cc-by
https://doaj.org/toc/2073-4433
https://www.mdpi.com/2073-4433/10/11/698/pdf,
https://hal.archives-ouvertes.fr/hal-02442585/document,
https://hal.archives-ouvertes.fr/hal-02442585,
https://academic.microsoft.com/#/detail/2984436684
http://dx.doi.org/10.3390/atmos10110698
under the license https://creativecommons.org/licenses/by/4.0/
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Published on 01/01/2019

Volume 2019, 2019
DOI: 10.3390/atmos10110698
Licence: Other

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